Metal Gear Solid 4 - Rex vs Ray fight
Arkham Asylum - When you get the chance to go Predator on a room full of mooks and get to hear them freak out as they find more and more bodies of their buddies and never see you.
Fallout 3 - Liberty Prime
Freedom Fighters - storming the Soviet news channel
Prototype - the first time I was able to do the dive bomb attack into Times Square and hitting a packed intersection
Okami - the boss fights especially the fight against the clockwork owls
Shadow of the Colossus - all of the colossi really. the sword-swinger was awesome, but the two fliers and the final colossus were my favorites
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Slightly off-kilter
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