First off I don't recommend the Ratchet & Clank and Jak & Daxter games made specifically for PSP (outsourcing to a different developer means you might as well set your franchise on fire).
Legend of Heroes: Trails in the Sky is a very interesting JRPG that shakes up a lot of the classic turn-based system and has so much style to it.
Most everything else I play and like has showed up already, but keep an eye out since they're adding more and more PSP games and with cross-play more and more PS3 releases will have a PSV version.
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